A global dust emission dataset for estimating dust radiative forcings in climate models

Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, Erik Kluzek

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

Sedimentary records indicate that atmospheric dust has increased substantially since preindustrial times. However, state-of-the-art global Earth system models (ESMs) are unable to capture this historical increase, posing challenges in assessing the impacts of desert dust on Earth's climate. To address this issue, we construct a globally gridded dust emission dataset (DustCOMMv1) spanning 1841-2000. We do so by combining 19 sedimentary records of dust deposition with observational and modeling constraints on the modern-day dust cycle. The derived emission dataset contains interdecadal variability of dust emissions as forced by the deposition flux records, which increased by approximately 50 % from 1851-1870 to 1981-2000. We further provide future dust emission datasets for 2000-2100 by assuming three possible scenarios for how future dust emissions will evolve. We evaluate the historical dust emission dataset and illustrate its effectiveness in enforcing a historical dust increase in ESMs by conducting a long-term (1851-2000) dust cycle simulation with the Community Earth System Model (CESM2). The simulated dust depositions are in reasonable agreement with the long-term increase in most sedimentary dust deposition records and with measured long-term trends in dust concentration at sites in Miami and Barbados. This contrasts with the CESM2 simulations using a process-based dust emission scheme and with simulations from the Coupled Model Intercomparison Project (CMIP6), which show little to no secular trends in dust deposition, concentration, and optical depth. The DustCOMM emissions thus enable ESMs to account for the historical radiative forcings (RFs), including due to dust direct interactions with radiation (direct RF). Our CESM2 simulations estimate a 1981-2000 minus 1851-1870 direct RF of -0.10 W m-2 by dust aerosols up to 10 μm in diameter (PM10) at the top of atmosphere (TOA). This global dust emission dataset thus enables models to more accurately account for historical aerosol forcings, thereby improving climate change projections such as those in the Intergovernmental Panel on Climate Change (IPCC) assessment reports.

Original languageEnglish
Pages (from-to)2311-2331
Number of pages21
JournalAtmospheric Chemistry and Physics
Volume25
Issue number4
DOIs
StatePublished - Feb 21 2025
Externally publishedYes

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