Measurement report: Airborne measurements of NOx fluxes over Los Angeles during the RECAP-CA 2021 campaign

Clara M. Nussbaumer, Bryan K. Place, Qindan Zhu, Eva Y. Pfannerstill, Paul Wooldridge, Benjamin C. Schulze, Caleb Arata, Ryan Ward, Anthony Bucholtz, John H. Seinfeld, Allen H. Goldstein, Ronald C. Cohen

Research output: Contribution to journalArticlepeer-review

9 Scopus citations

Abstract

Nitrogen oxides (NOxNO+NO2) are involved in most atmospheric photochemistry, including the formation of tropospheric ozone (O3). While various methods exist to accurately measure NOx concentrations, it is still a challenge to quantify the source and flux of NOx emissions. We present airborne measurements of NOx and winds used to infer the emission of NOx across Los Angeles. The measurements were obtained during the research aircraft campaign RECAP-CA (Re-Evaluating the Chemistry of Air Pollutants in CAlifornia) in June 2021. Geographic allocations of the fluxes are compared to the NOx emission inventory from the California Air Resources Board (CARB). We find that the NOx fluxes have a pronounced weekend effect and are highest in the eastern part of the San Bernardino Valley. The comparison of the RECAP-CA and the modeled CARB NOx fluxes suggests that the modeled emissions are higher than expected near the coast and in Downtown Los Angeles and lower than expected further inland in the eastern part of the San Bernardino Valley.

Original languageEnglish
Pages (from-to)13015-13028
Number of pages14
JournalAtmospheric Chemistry and Physics
Volume23
Issue number20
DOIs
StatePublished - Oct 16 2023
Externally publishedYes

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