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Multi-Species Constraints Resolve Methane Source Versus Sink Changes: Lessons From 2020

  • Xueying Yu
  • , Dylan B. Millet
  • , Daven K. Henze
  • , Helen Worden
  • , Corinne Vigouroux
  • , Prabir Patra
  • , Jason D. Hill
  • , Robert B. Jackson
  • SUNY Albany
  • University of Minnesota Twin Cities
  • Stanford University
  • University of Colorado Boulder
  • National Center for Atmospheric Research
  • Royal Belgian Institute for Space Aeronomy
  • Japan Agency for Marine-Earth Science and Technology
  • Department of Bioproducts and Biosystems Engineering

Research output: Contribution to journalArticlepeer-review

Abstract

Satellite observations show that atmospheric methane (CH4) increased by a record-breaking 19 ppb in 2020, but the causes are unclear because of uncertain impacts from COVID-related pollutant shifts on hydroxyl (OH) radical concentrations. Here we employ an ensemble of constraints to simultaneously quantify methane sources and sinks for 2020 in a manner consistent with space-based measurements of its oxidation products (formaldehyde, HCHO; carbon monoxide, CO) and with in situ measurements of methyl chloroform (MCF, an OH proxy). We find that resolving methane source and sink changes requires constraints from the CH4-HCHO-CO cascade and from MCF: reliance on either alone causes overfitting. The optimized year-2020 global methane sources (557 [514–601] Tg/y) and sinks (505 [459–550] Tg/y) are at the low end of Global Carbon Project ensemble estimates. We further resolve the 2020 methane increase into two distinct periods. During March-May, inversions reveal that methane emissions and global-mean OH values are both lower than predicted; the latter likely reflects offsetting impacts from methane and other pollutants. From June-August, inversions identify methane emission underestimates that mainly reflect temperature-driven biogenic sources. Our study highlights the methane lifetime increase that can accompany reduced pollutant emissions, and demonstrates the necessity of multi-species, satellite-based observations for understanding and attributing future methane trends.

Original languageEnglish
Article numbere2025EF007067
JournalEarth's Future
Volume14
Issue number6
DOIs
StatePublished - Jun 2026
Externally publishedYes

Keywords

  • Methane emissions
  • OH
  • atmospheric oxidation
  • inverse analysis
  • multi-species

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